Soft robots have demonstrated exceptional potential in various applications, particularly in biomedicine, which is attributed to their motional agility and machinability. However, their potential applications in water remediation have not been fully explored. The main challenge is to achieve both precise motion and efficient pollutant degradation. Herein, a modular design is reported for fabricating soft robots. These robots are designed with spatially separated components. One is superparamagnetic iron oxide nanoparticles for magnetic actuation and the other is photocatalysts for targeted pollutant degradation (i.e., methyl orange, congo red, rhodamine B, tetracycline, and soybean oil). The helical structure enables diverse programmable motional modes, including high-speed propulsion up to 3.54 mm s