In Silico Characterization of Glycan Ions from IM-MS Collision Cross Section.

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Tác giả: Mithony Keng, Kenneth M Merz

Ngôn ngữ: eng

Ký hiệu phân loại: 606 Organizations

Thông tin xuất bản: United States : Journal of the American Society for Mass Spectrometry , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 15179

Ion mobility mass spectrometry (IM-MS) can assist in the identification of isobaric chemical analytes by exploiting the difference in their gas phase collision cross-section (CCS) property. In glycomics, reliable glycan characterization remains challenging, even with IM-MS, because of closely related isomeric species and the available binding arrangements of substituted monosaccharides, allowing for the formation of complex structures. Here, we present a computational procedure to obtain gas-phase structural information from the experimental IM-MS CCS data of carbohydrates. The workflow proceeds with high throughput charge modeling of glycan seed structures to determine the precise protonation or deprotonation site. The charge models were then screened by using density functional theory (DFT) to produce candidate charge states for conformation generation. An extensive conformational scoring of the glycan ions was performed quantum mechanically at the DFT D3-B3LYP/6-31G+(d,p) level for the negative mode, [M - H]
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