Discovery of a novel C2-functionalized chromen-4-one scaffold for the development of p38α MAPK signaling inhibitors to mitigate neutrophilic inflammatory responses.

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Tác giả: Yi-Han Chang, Po-Jen Chen, Shun-Hua Chen, Tzu-Peng Cheng, Ching-Ho Chi, Shu-Yen Fang, Hsin-Yi Hung, Yi-Chen Lee, Keng-Chang Tsai

Ngôn ngữ: eng

Ký hiệu phân loại: 028.108 Reviews with respect to kinds of persons

Thông tin xuất bản: England : Biochemical pharmacology , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 164723

Neutrophil dysregulation is implicated in a spectrum of inflammatory pathologies, suggesting the potential for targeting neutrophilic hyperactivation as a pharmacological strategy to manage inflammatory disorders. Building upon prior research where 2-thiolphenoxychromone derivatives were found to inhibit neutrophilic generation of superoxide anions, this study focused on exploring the structure-activity relationship (SAR) of different C2 bridging moieties and anti-inflammatory effects using bioisosteric replacements and scaffold-hopping approaches. Among various chemotypes, the N-(4-oxo-4H-chromen-2-yl)benzenesulfonamide derivatives emerged as robust inhibitors of both superoxide anion generation and elastase release from fMLF-activated human neutrophils, with IC
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