Self-remodeling material can change their physical properties based on mechanical environment. Recently, mechanically controlled polymerization using mechanoredox catalyst enabled composite materials to undergo a permanent structural change, thereby enhancing their mechanical strength. However, a significant delay in material's response was observed due to the sluggish activation of the bulk catalyst for polymerization. Herein, we report a fast, mechanically controlled radical polymerization of water soluble monomers using 2D MoS