Novel supramolecular artificial light-harvesting systems based on AIE-active macrocycles for efficient white-light photocatalysis in water.

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Tác giả: Ke Chen, Hai-Tao Feng, Chunxuan Qi, Ben Zhong Tang, Jun-Cheng Yang, Guo-Ling Zhang

Ngôn ngữ: eng

Ký hiệu phân loại: 341.733 +Disarmament

Thông tin xuất bản: England : Chemical science , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 171496

Constructing supramolecular artificial light-harvesting systems (ALHSs) based on the Förster resonance energy transfer (FRET) mechanism provides an optimal platform for understanding natural photosynthesis and simulating natural light-harvesting systems. In the present work, rigid macrocycle K-1 with a nonplanar conformation and aggregation-induced emission (AIE) properties was selected as an energy donor in ALHSs, while the non-cyclic AIEgen K-2 was used for a comparative study. In aqueous solution, an efficient one-step energy-transfer process was established between blue-emitting K-1 and an acceptor (namely PBTB) with orange fluorescence to afford a high energy-transfer efficiency (
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