Design, Synthesis, and Biological Evaluation of BODIPY-Caged Resiquimod as a Dual-Acting Phototherapeutic.

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Tác giả: Manabu Abe, Ismail Celik, Yasuhiro Ishihara, Yutaka Kikuchi, Elsayed S I Mohammed, Norimitsu Morioka, Yoki Nakamura, Eslam Roshdy, Haruko Takahashi, Haruto Taniguchi

Ngôn ngữ: eng

Ký hiệu phân loại: 519.57 Design of experiments

Thông tin xuất bản: United States : Journal of medicinal chemistry , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 180410

Resiquimod, an imidazoquinoline scaffold, exhibits potent immunotherapeutic activity but is associated with off-target effects, limiting its clinical utility. To address this limitation, we developed a novel BODIPY-caged resiquimod that is responsive to red light, combining photocaging and photodynamic therapy functionalities. Molecular docking studies guided identification of the optimal caging site for resiquimod, effectively masking its immune activity. BODIPY-caged resiquimod remained inactive under dark conditions, effectively masking resiquimod's immunostimulatory effects. However, red light irradiation precisely uncaged resiquimod, inducing robust immune activation, even in the presence of
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