Short-Side-Chain Membranes with Stabilized Superacid on Graphitic Carbon Nitride for Polymer Electrolyte Fuel Cells under Low-Humidity Conditions.

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Tác giả: Santoshkumar D Bhat, Maniprakundil Neeshma, Punnappadam Rajan Suraj

Ngôn ngữ: eng

Ký hiệu phân loại: 297.1248 Sources of Islam

Thông tin xuất bản: United States : ACS applied materials & interfaces , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 180961

The integration of superacid-like heteropolyacids offers a promising route to develop highly proton-conducting membranes for energy storage and conversion. However, the inherent hydrophilicity of these acids can cause leaching, which undermines the fuel cell performance. In our research, we engineered a proton-conductive membrane with a facile hydrothermal synthesis approach to form stabilized hybrid superacids, namely, phosphotungstic acid (PTA), with graphitic carbon nitride (PCN) and its incorporation in a short-side-chain ionomer, namely, Aquivion. This unique approach via PCN nanohybrids enhances the proton transport within the membrane. These nanohybrids effectively combined the strong acidity of PTA with continuous 2D proton-transport pathways via a short side chain, resulting in a notable proton conductivity of 0.228 S cm
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