Layer-dependent evolution of electronic structures and correlations in rhombohedral multilayer graphene.

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Tác giả: Hao Cai, Tongtong Chen, Lin He, Yuanyuan Hu, Lei Liao, Wei-Yu Liao, Xingqiang Liu, Zhihui Qin, Ya-Ning Ren, Qiwei Tian, Yuan Tian, Ling-Hui Tong, Wen-Xiao Wang, Yiliu Wang, Si-Min Xue, Long-Jing Yin, Chen Zhang, Li Zhang, Lijie Zhang, Shihao Zhang, Yang Zhang, Yue-Ying Zhou, Ruo-Jue Zou, Xuming Zou

Ngôn ngữ: eng

Ký hiệu phân loại: 271.6 *Passionists and Redemptorists

Thông tin xuất bản: England : Nature nanotechnology , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 188233

The recent discovery of superconductivity and magnetism in trilayer rhombohedral graphene (RG) establishes an ideal, untwisted platform to study strong correlation electronic phenomena. However, the correlated effects in multilayer RG have received limited attention, and, particularly, the evolution of the correlations with increasing layer number remains an unresolved question. Here we show the observation of layer-dependent electronic structures and correlations-under surprising liquid nitrogen temperature-in RG multilayers from 3 to 9 layers by using scanning tunnelling microscopy and spectroscopy. We explicitly determine layer-enhanced low-energy flat bands and interlayer coupling strengths. The former directly demonstrates the further flattening of low-energy bands in thicker RG, and the latter indicates the presence of varying interlayer interactions in RG multilayers. Moreover, we find significant splittings of the flat bands, ranging from ~50 meV to 80 meV, at 77 K when they are partially filled, indicating the emergence of interaction-induced strongly correlated states. Particularly, the strength of the correlated states is notably enhanced in thicker RG and reaches its maximum in the six-layer, validating directly theoretical predictions and establishing abundant new candidates for strongly correlated systems. Our results provide valuable insights into the layer dependence of the electronic properties in RG and demonstrate it as a suitable system for investigating robust and highly accessible correlated phases.
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