Improvement of shear strength of starch-based wood adhesives using polysilsesquioxane/polyvinyl acetate hybrid nanoparticles.

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Tác giả: Ali Ahmadi-Dehnoei, Somayeh Ghasemirad, Parisa Shahabi-Sirmandi

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: Netherlands : International journal of biological macromolecules , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 195145

An environmentally friendly wood adhesive for use in indoor applications was prepared by blending polymethacryloxypropylsilsesquioxane (PSQ)/polyvinyl acetate (PVAc) hybrid nanoparticles (HNPs) and a starch-based wood adhesive. HNPs were synthesized by emulsion polymerization of vinyl acetate in the presence of PSQ core nanoparticles, and then added in various amounts to a starch-based wood adhesive, prepared by grafting of PVAc onto starch. Energy-dispersive X-ray analysis coupled with field-emission scanning electron microscopy revealed uniform dispersion and distribution of HNPs in the composite adhesives due to compatibility of the PVAc shell with the PVAc-grafted starch. The addition of HNPs improved the film-forming ability of the adhesive and alleviated the agglomeration of starch. It also improved the adhesives toughness, appeared with multiple shear bands in their cross-sectional microscopic images. Thus, inclusion of 3, 7, and 20 wt% HNP into the adhesive resulted in 50, 65, and 74 % improvement in its dry shear strength, respectively. However, the excessive increase in the viscosity of the adhesive containing 30 wt% HNP reduced its dry shear strength to a value similar to that of the pristine adhesive. The increase in the HNPs content from 7 to 30 wt% improved the thermal stability of the adhesives.
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