Shear-induced dynamics of an active Belousov-Zhabotinsky droplet.

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Tác giả: Kvs Chaithanya, Pratyush Dayal, Shreyas A Shenoy

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: England : Soft matter , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 208878

Controlled navigation of self-propelled active matter in complex biological environments has remained a significant challenge in engineering owing to a multitude of interactions that persist in the process. Active droplets, being some of the several synthetic active matters, have garnered significant attention owing to their ability to exhibit dynamic shape changes, self-sustained motion, interact with external stimuli such as flows, and mimic biological active matter. Here, we explore the dynamics of a self-propelled active droplet powered by the oscillatory Belousov-Zhabotinsky (BZ) reaction in the presence of a shear flow. We adapt a multicomponent lattice Boltzmann method (LBM) in conjunction with the phase-field model to simulate the droplet's interaction with the surrounding fluid. We unravel the collective effect of droplet deformation, reaction kinetics, and strength of the surrounding shear flow on droplet dynamics. Our findings depict that the shear flow disrupts the initial isotropic surface tension, and produces concentration nucleation spots in the droplet. The asymmetry thus generated produces Marangoni flow that ultimately propels the droplet. Our findings provide valuable insights into the mechanisms governing active droplet behavior and open new avenues for designing controllable synthetic active matter systems with potential applications in microfluidics, targeted delivery, and biomimetic technologies. In addition, our framework can potentially be integrated with the physics-informed machine learning framework to develop more efficient mesh-free methods.
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