New synthetic pathway towards BTrzPhen-tetraol: a hydrophilic 2,9-bis-triazolyl-1,10-phenanthroline ligand for selective americium stripping.

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Tác giả: T Cardinaels, W Dehaen, T Opsomer, F Reniers, P Troosters, K Van Hecke, K Van Hoecke, K Verguts, P Zsabka

Ngôn ngữ: eng

Ký hiệu phân loại: 297.1248 Sources of Islam

Thông tin xuất bản: England : Dalton transactions (Cambridge, England : 2003) , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 208980

Selectively separating Am(III) from nuclear waste streams is an extremely challenging task due to the presence of the trivalent lanthanides and Cm(III). 1,10-Phenanthroline ligands decorated with 1,2,4-triazines or 1,2,3-triazoles have emerged as promising extractants for achieving such separation. In this article, a new robust synthetic pathway towards the hydrophilic, CHON compliant bistriazoylphenanthroline ligand BTrzPhen-tetraol is reported. BTrzPhen-tetraol was synthesised both as the hydrochloride and as a free base with overall yields of 66% and 48%, respectively. The ligand demonstrated excellent solubility and stability in dilute nitric acid solutions, with no observable decomposition after three days in 0.5 mol L
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