Super Bending-Stable Flexible Colloidal QD Photodetector with Fast Response and Near-Unity Carrier Extraction Efficiency.

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Tác giả: Jing Bai, Yu-Hao Deng, Pieter Geiregat, Zeger Hens, Ezat Kheradmand, Itai Lieberman, Chao Pang, Abu Bakar Siddik, Dries Van Thourhout

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: United States : ACS applied materials & interfaces , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 214566

Flexible colloidal quantum dot (QD) optoelectronics apply the superior properties of colloidal QDs to flexible devices, exhibiting unique advantages in the fields of imagers, solar cells, displays, wearable sensors, on-skin electronics, robotics, and bioimaging. Here, we show that colloidal QD photodiodes (QDPDs) with an ultrathin QD absorber layer have record bending stability with 100,000 repetitive bending cycles in QD devices. The QDPDs obtained a high-quality p-n junction with a 1700 rectification ratio. The formation of a Fabry-Pérot cavity by the layered stack results in a 3.4-fold enhanced light absorption, while the ultrathin structure ensures a near-unity efficient extraction (97%) of photogenerated charge carriers from the PbS QD film upon illumination with 1330 nm short-wavelength infrared light. Finally, upon suppression of the capacitance effect, the response time of this QDPD can be as short as 20 ns, which is the fastest response for flexible colloidal QDPDs.
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