The discovery of a random endo-acting ι-carrageenase with bifunctional activities against ι-carrageenan and κ-carrageenan.

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Tác giả: Yaoguang Chang, Fangyi Chen, Guangning Chen, Xuanwei Mei, Jingjing Shen, Changhu Xue, Yuying Zhang, Long Zheng, Jinhang Zhou

Ngôn ngữ: eng

Ký hiệu phân loại: 271.6 *Passionists and Redemptorists

Thông tin xuất bản: Netherlands : International journal of biological macromolecules , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 216576

Carrageenans have attracted increasing research interests in recent decades for their various physicochemical and physiological properties. Random endo-acting carrageenases are promising tools for tailoring the molecular weight of carrageenan and preparing a series of carrageenan oligosaccharides. Although the processive ι-carrageenases in the GH82 family have been widely investigated, the random ι-carrageenase has not been reported. Herein, a novel GH82 family protein Cg82Mf, which was identified by AlphaFold2 as lacking a lid structure on the catalytic groove, was cloned and expressed in Escherichia coli. The analysis of hydrolysis pattern proved that Cg82Mf was the first random endo-acting enzyme against ι-carrageenan, and was capable of preparing the hydrolysis products with various degrees of polymerization. Cg82Mf exhibited higher substrate affinity among all characterized ι-carrageenases, reflected by its low K
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