Explore the toxicological mechanism of 6PPD-Q on human health through a novel perspective: The interaction between lactate dehydrogenase and 6PPD-Q.

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Tác giả: Zhengjiang Fu, Zimeng He, Lin Kuang, Jiaqing Luo, Xun Tuo, Xiaowei Wang, Wei Zhang, Yue Zhang

Ngôn ngữ: eng

Ký hiệu phân loại: 271.6 *Passionists and Redemptorists

Thông tin xuất bản: Netherlands : International journal of biological macromolecules , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 216672

N-(1,3-dimethylbutyl)-N'-phenyl-p-phenylenediamine-quinone (6PPD-Q), an oxidative derivative of tire anti-degradant, has been linked to mortality in coho salmon (Oncorhynchus kisutch) and has exhibited potential human toxicity. Hence, exploring how 6PPD-Q interacts with biomacromolecules like enzymes is indispensable to assess its human toxicity and elucidate its mechanism of action. This investigation aims to explore the impact of 6PPD-Q on lactate dehydrogenase (LDH) through various methods. The findings indicate that 6PPD-Q can spontaneously embed in the coenzyme site of LDH and obviously change the biological activity of LDH by non-competitive inhibition. Simultaneously, this inhibitory effect is concentration-dependent. 6PPD-Q can affect both the level of LDH and the transcription of Ldha in AML-12 cells. Hydrogen bonding and van der Waals forces serve as the primary driving forces in LDH-6PPD-Q combination process. The apparent binding constant (K
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