Site-Specific Competitive Kinase Inhibitor Target Profiling Using Phosphonate Affinity Tags.

 0 Người đánh giá. Xếp hạng trung bình 0

Tác giả: Marc P Baggelaar, Albert J R Heck, Anneroos E Nederstigt, Wouter van Bergen

Ngôn ngữ: eng

Ký hiệu phân loại: 617.76 Diseases of ocular neuromuscular mechanism and lacrimal apparatus

Thông tin xuất bản: United States : Molecular & cellular proteomics : MCP , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 217367

Protein kinases are prime targets for drug development due to their involvement in various cancers. However, selective inhibition of kinases, while avoiding off-target effects remains a significant challenge for the development of protein kinase inhibitors. Activity-based protein profiling (ABPP), in combination with pan-kinase activity-based probes (ABPs) and mass spectrometry-based proteomics, enables the identification of kinase drug targets. Here, we extend existing ABPP strategies for kinase profiling with a site-specific analysis, allowing for protein kinase inhibitor target engagement profiling with amino acid specificity. The site-specific approach involves highly efficient enrichment of ABP-labeled peptides, resulting in a less complex peptide matrix, straightforward data analysis, and the screening of over ∼100 kinase active sites in a single LC-MS analysis. The complementary use of both trypsin and pepsin in parallel to generate the ABP-labeled peptides considerably expanded the coverage of kinases and pinpoint the exact binding sites. Using the site-specific strategy to examine the on- and off-targets of the Ephrin receptor (Eph) B4 inhibitor NVP-BHG712 showed binding to EphA2 with an IC
Tạo bộ sưu tập với mã QR

THƯ VIỆN - TRƯỜNG ĐẠI HỌC CÔNG NGHỆ TP.HCM

ĐT: (028) 36225755 | Email: tt.thuvien@hutech.edu.vn

Copyright @2024 THƯ VIỆN HUTECH