Peripheral Modification Strategy of Heavy Atom for High-Performance Multi-Resonance Thermally Activated Delayed Fluorescence Emitters.

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Tác giả: Zhuang Cheng, Yixuan Jiang, Futong Liu, Ping Lu, Xiaobo Ma, Zihan Su, Liang Wan, Yan Yan, Zhenyu Yan

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: Germany : Chemistry (Weinheim an der Bergstrasse, Germany) , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 218747

Organic light-emitting materials with multi-resonance thermally activated delayed fluorescence (MR-TADF) have shown great potential for realizing highly efficient narrowband organic light-emitting diodes (OLEDs). However, the heavy efficiency roll-off caused by the slow reverse intersystem crossing (RISC) process remains a challenging issue for the further practical application of MR-TADF materials. Here, we develop two TADF emitters, BNDBT and BNDBF, in which the dibenzothiophene and dibenzofuran substituents are attached at the bottom of the B/N frameworks. They all exhibit the similar high photoluminescence quantum yields of 90 % and 87 %. The sulfur-containing material BNDBT exhibits a RISC rate (k
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