Imaging the Photochemistry of the Hydrogen-Bonded Heptazine-Water Complex with Femtosecond Time-Resolved Spectroscopy: A Computational Study.

• Tác giả: Lipeng Chen, Wolfgang Domcke, Maxim F Gelin, Sebastian V Pios
• Ngôn ngữ: eng
• Ký hiệu phân loại: 171.8 Systems based on altruism
• Thông tin xuất bản: United States : The journal of physical chemistry. A , 2025
• Bộ sưu tập: NCBI
• ID: 220225

Tóm tắt

Graphitic carbon nitride (g-CN) has attracted vast interest as a promising inexpensive metal-free photocatalyst for water splitting with solar photons. The heptazine (Hz) molecule is the building block of graphitic carbon nitride. The photochemistry of the Hz molecule and derivatives thereof in protic environments has been the subject of several recent experimental and computational studies. In the present work, the hydrogen-bonded Hz···H