With the advancement of artificial intelligence (AI), many AI-derived techniques have been adapted into psychological and behavioral science research, including measure development, which is a key task for psychometricians and methodologists. Ant colony optimization (ACO) is an AI-derived metaheuristic algorithm that has been integrated into the structural equation modeling framework to search for optimal (or near optimal) solutions. ACO-driven measurement modeling is an emerging method for constructing scales, but psychological researchers generally lack the necessary understanding of ACO-optimized models and outcome solutions. This article aims to investigate whether ACO solutions are indeed optimal and whether the optimized measurement models of ACO are always more psychologically useful compared to conventional ones built by human psychometricians. To work toward these goals, we highlight five essential methodological considerations for using ACO in measure development: (a) pursuing a local or global optimum, (b) avoiding a subjective optimum, (c) optimizing content validity, (d) bridging the gap between theory and model, and (e) recognizing limitations of unidirectionality. A joint data set containing item-level data from German (