Tuning the Stability of DNA Tetrahedra with Base Stacking Interactions.

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Tác giả: Jibin Abraham Punnoose, Arun Richard Chandrasekaran, Alan A Chen, Dadrian Cole, Ken Halvorsen, Bharath Raj Madhanagopal, Tristan Melfi, Vinod Morya, Sweta Vangaveti

Ngôn ngữ: eng

Ký hiệu phân loại: 671.520422 Joining and cutting of metals

Thông tin xuất bản: United States : Nano letters , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 229783

DNA nanotechnology uses the programmable assembly of DNA to create nanoscale objects. Recent work from our laboratory suggested that terminal stacking interactions between adjacent strands could be a design parameter for DNA nanotechnology. Here, we explore that idea by creating DNA tetrahedra with sticky ends containing identical base pairing interactions but different stacking interactions. Testing all 16 stacking combinations, we found that the melting temperature of DNA tetrahedra varied by up to 10 °C from altering a single base stack in the design. We also show that a 4 bp sticky end with weak stacking does not form stable tetrahedra, while strengthening the stacks confers high stability with a 46.8 ± 1.2 °C melting temperature, comparable to that of a 6 bp sticky end with weak stacking (49.7 ± 2.9 °C). The results likely apply to other DNA nanostructures and suggest that stacking interactions play a role in the formation and stability of DNA nanostructures.
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