Intracellular dehydrogenation catalysis leads to reductive stress and immunosuppression.

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Tác giả: Xiaoming Cai, Chunying Chen, Xingfa Gao, Jie Jiang, Ruibin Li, Xi Liu, Xinlian Wang, Zhenzhen Wang, Qianqian Xie, Qing Yang, Huizhen Zheng

Ngôn ngữ: eng

Ký hiệu phân loại: 296.1138 Sources

Thông tin xuất bản: England : Nature nanotechnology , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 232627

Imbalanced redox homeostasis, involving either oxidative stress or reductive stress, can profoundly impact cellular functions, contributing to various diseases. While the implications of oxidative stress in the adverse effects of nanoparticles have been extensively studied, our comprehension of reductive stress within the context of nano-redox system interactions remains limited. Here we illuminate a domino effect initiated by the dehydrogenase-like activity of transition metal borides. Specifically, seven transition metal borides were identified to emulate the enzymatic activity of natural dehydrogenases, resulting in heightened levels of reductive constituents within critical biological redox pairs in cells. Mass cytometry analysis provides compelling evidence that reductive stress initiates an immunosuppressive environment within lung tissues, promoting the metastasis of breast cancer cells to the lungs. In summary, our study unveils the chemical basis of nano-induced reductive stress and establishes a mechanistic axis that interlinks dehydrogenase-like activity, reductive stress, immunosuppression and tumour metastasis.
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