Wood-based hydrogel with a unique anisotropic structure is an attractive soft-and-wet material. However, it remains a challenge to simultaneously achieve robust, multi-functional, and multi-response integrations through a sustainable and green approach. Herein, a bioinspired, additive-free method is reported to fabricate composite hydrogels reinforced by naturally high-strength wood skeleton without using any chemical initiators and crosslinking agents. Specifically, polymers (Polyacrylamide/Polyacrylic acid) are grafted from the surfaces of the aligned cellulose of wood skeleton, forming wood-based hydrogels under UV irradiation. Afterward, Fe