Bottlebrush block copolymers (BBCPs), characterized by densely grafted side chains along their backbone, have emerged as promising materials for structural color applications. Their unique architecture prevents entanglement and facilitates rapid assembly kinetics, enabling the formation of various photonic crystals with high tunability of structural color from the visible to the infrared range. However, accessing non-1D structures has been largely limited to synthetic approaches. In this paper, we report large modulation of a microphase separated morphology of the polystyrene-