Electron bifurcation [electronic resource] : progress and grand challenges

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Tác giả:

Ngôn ngữ: eng

Ký hiệu phân loại: 541.38 Radiochemistry

Thông tin xuất bản: Washington, D.C. : Oak Ridge, Tenn. : United States. Dept. of Energy. Office of Science ; Distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, 2019

Mô tả vật lý: Size: p. 11823-11832 : , digital, PDF file.

Bộ sưu tập: Metadata

ID: 262753

 Electron bifurcation moves electrons from a two-electron donor to reduce two spatially separated one-electron acceptors. If one of the electrons reduces a high-potential (lower energy) acceptor, then the other electron may proceed ?uphill? to reduce a low-potential (higher energy) acceptor. This mechanism is now considered the third mode of energy transduction in biology, and offers promise for the development of novel bioinspired energy conversion strategies. Nature uses electron bifurcation to realize highly sought-after reactions: reversible CO<
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  reduction, nitrogen fixation, and hydrogen production. In this review, we summarize the current understanding of electron bifurcation, including both recent progress and outstanding questions in understanding and developing artificial EB systems.
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