Chemical-Looping Combustion and Gasification of Coals and Oxygen Carrier Development [electronic resource] : A Brief Review

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Tác giả:

Ngôn ngữ: eng

Ký hiệu phân loại: 622.33 *Carbonaceous materials

Thông tin xuất bản: Morgantown, W.Va. : Oak Ridge, Tenn. : National Energy Technology Laboratory (U.S.) ; Distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, 2015

Mô tả vật lý: Size: p. 10605-10635 : , digital, PDF file.

Bộ sưu tập: Metadata

ID: 263590

 Chemical-looping technology is one of the promising CO<
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  capture technologies. It generates a CO<
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  enriched flue gas, which will greatly benefit CO<
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  capture, utilization or sequestration. Both chemical-looping combustion (CLC) and chemical-looping gasification (CLG) have the potential to be used to generate power, chemicals, and liquid fuels. Chemical-looping is an oxygen transporting process using oxygen carriers. Recently, attention has focused on solid fuels such as coal. Coal chemical-looping reactions are more complicated than gaseous fuels due to coal properties (like mineral matter) and the complex reaction pathways involving solid fuels. The mineral matter/ash and sulfur in coal may affect the activity of oxygen carriers. Oxygen carriers are the key issue in chemical-looping processes. Thermogravimetric analysis (TGA) has been widely used for the development of oxygen carriers (e.g., oxide reactivity). Two proposed processes for the CLC of solid fuels are in-situ Gasification Chemical-Looping Combustion (iG-CLC) and Chemical-Looping with Oxygen Uncoupling (CLOU). The objectives of this review are to discuss various chemical-looping processes with coal, summarize TGA applications in oxygen carrier development, and outline the major challenges associated with coal chemical-looping in iG-CLC and CLOU.
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