Morphology and mixing state of individual freshly emitted wildfire carbonaceous particles [electronic resource]

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Tác giả:

Ngôn ngữ: eng

Ký hiệu phân loại: 363.738 Pollutants

Thông tin xuất bản: Washington, D.C. : Oak Ridge, Tenn. : United States. Dept. of Energy. Office of Science ; Distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, 2013

Mô tả vật lý: Size: Article No. 2122 : , digital, PDF file.

Bộ sưu tập: Metadata

ID: 263867

 Biomass burning is one of the largest sources of carbonaceous aerosols in the atmosphere, significantly affecting earth?s radiation budget and climate. Tar balls, abundant in biomass burning smoke, absorb sunlight and have highly variable optical properties, typically not accounted for in climate models. Here we analyse single biomass burning particles from the Las Conchas fire (New Mexico, 2011) using electron microscopy. We show that the relative abundance of tar balls (80%) is 10 times greater than soot particles (8%). We also report two distinct types of tar balls
  one less oxidized than the other. Furthermore, the mixing of soot particles with other material affects their optical, chemical and physical properties. We quantify the morphology of soot particles and classify them into four categories: B50% are embedded (heavily coated), B34% are partly coated, B12% have inclusions andB4% are bare. Inclusion of these observations should improve climate model performances.
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