Dynamics of Thermally Driven Domain Transformation in Ferroelectric Thin Films.

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Tác giả: Matthew Dawber, Andrei Fluerasu, Anna Gura, Rui Liu, Theodore Sauyet, Lutz Wiegart, Yugang Zhang

Ngôn ngữ: eng

Ký hiệu phân loại: 530.4275 States of matter

Thông tin xuất bản: United States : Physical review letters , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 474077

An important feature in ultrathin ferroelectric films is the spontaneous formation of nanoscale polarization domain patterns. Epitaxial strain can greatly increase the ferroelectric transition temperature such that films can be in the ferroelectric state during growth. On the other hand, depolarization fields compete with ferroelectricity in ultrathin films, and, consequently, the optimal domain configuration during growth is a moving target. Under these conditions it is readily possible for a grown film to be in a nonequilibrium domain configuration. As the energy landscape in the system is quite complex, the relaxation dynamics by which a system can evolve towards the true equilibrium configuration are also quite interesting. To capture the details of this process we used Bragg-geometry x-ray photon correlation spectroscopy (XPCS), in which x-ray scattering speckle patterns contain the information from the domain arrangements inside the film. With modest heating (∼150 °C) domain relaxation from T (tetragonal) to M_{C} (monoclinic) was observed in BaTiO_{3} films grown on ultrathin ferroelectric PbTiO_{3} layers. Two-time correlation analysis reveals fascinating details associated with sticking points and reversals in the process.
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