Electron-Withdrawing Hexagonal Boron Nitride as a Biocompatible and Metal-Free Antibacterial Platform.

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Tác giả: Yichao Bai, Jianxiang Gao, Haoqi He, Feiyu Kang, Yu Lei, Wenbo Li, Xudong Liu, Lan Ma, Vijay Pandey, Linxuan Sun, Mauricio Terrones, Hengyue Xu, Qiangmin Yu, Xi Zhang, Mingchuang Zhao, Yingcan Zhao

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: United States : Nano letters , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 489347

 Inert hexagonal boron nitride (h-BN) is a prominent two-dimensional material known for its wide bandgap, thermal stability, and biocompatibility, but it resists functionalization due to strong B-N bonds. This study presents a method to fluorinate h-BN via cryomilling, resulting in ∼30 atom % fluorine loading (F-dBN). This modification prevents the formation of C-F bonds associated with adverse health effects, enhances biocompatibility, and introduces electron-withdrawing properties that improve the material's chemical reactivity and antibacterial efficiency while significantly reducing its bandgap from 5.77 to 3.64 eV. Using a microdroplet electrochemical setup, the charge transfer at the F-dBN-bacterium interface is amplified by osmotic pressure, showing that F moieties enhance extracellular electron transfer and disrupt bacterial charge balance. Notably, F-dBN exhibits >
 99% antibacterial activity against
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