Negatively charged organic pollutants in water are responsible for a large range of public health and ecological issues. Low-cost and low-toxicity graphitic carbon nitride (CN), with its abundant functional groups and surface defects, is a promising material for the removal of organic molecules by adsorption. However, basic synthesis methods for CN often result in a material with morphology and electric charge that are suboptimal for interacting with negatively charged pollutants. Here, an adsorbent was prepared by thermally oxidizing a tubular CN precursor and then coating the resulting flake-shaped material (FCNO) with the polycationic polymer polyethyleneimine (PEI). The resulting adsorbent, FCNO