The isolation of two terpenoids, named 1alpha,6beta-dihydroxy-4(l4)-eudesmene (1), niloticine (2), and two phenolic glucosides, dimethyl crenatin (3), and leonuriside A (4) trom the stem and root of Brucea mpllis Wall. ex Kurz, were reported. Their structures were elucidated on the basis of spectral data, including 1D, 2D NMR and MS.