Load-bearing fibrous tissues, like tendons, have remarkable strength with high water content (∼60%) due to the anisotropic network of collagen fibers. However, the scalability of biomimetic anisotropic hydrogels is limited by time-intensive fabrication processes involving cross-linking and stretching, often spanning several hours to days. Here, we present a rapid, scalable approach for fabricating tendon-mimetic hydrogel fibers within 1 min using the synergistic engineering of cyano-