Photogeneration and visualization of a surface-stabilized dinitrene.

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Tác giả: Jan Berger, Sofia Canola, Qifan Chen, Karl-Heinz Ernst, Federico Frezza, José María Gómez-Fernandez, Leonhard Grill, Pavel Jelinek, Jiří Klívar, José Ángel Martín-Gago, Pingo Mutombo, Christophe Nacci, Ana Sánchez-Grande, Carlos Sánchez-Sánchez, Irena G Stará, Ivo Starý

Ngôn ngữ: eng

Ký hiệu phân loại: 553.3 Iron

Thông tin xuất bản: Germany : Angewandte Chemie (International ed. in English) , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 663236

Nitrenes are known as key intermediates in various chemical reactions. Nitrene transfer reactions are particularly effective for synthesizing nitrogen-containing compounds, where metal catalysts play a crucial role in controlling nitrene reactivity and selectivity. In this study, we demonstrate the formation of a stable surface-supported dinitrene on Au(111) through UV irradiation of its diazide precursor, characterized by scanning probe techniques. The photoreaction mechanism is elucidated with wavelength-dependent experiments and time-dependent density functional theory calculations. Our findings present the first real-space visualization of a metal nitrene adsorbed on a surface, highlighting its potential in catalysis and surface functionalization.
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