Effectively Controlling NIR Emissive Property and the ESIPT Behavior of Modified Styryl Dyes by Atomic Substituent: DFT/TD-DFT Approach.

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Tác giả: Bhawna Pareek, Govindasami Periyasami, Selva Kumar Ramasamy, Dineshkumar Sengottuvelu, Shilpa Taneja, Geetha Venkatesan

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: Netherlands : Journal of fluorescence , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 676606

Recent literature on biosensing and bioimaging has explored excited state intramolecular proton transfer (ESIPT) cyanide dyes. These classes of fluorescence dyes generally use the classical pyridinium or indolium cations acceptor units' styrene with the ESIPT core. This work studied the photophysical and ESIPT kinetics of novel flavylium cation as an acceptor unit styrene with an ESIPT core using DFT/TD-DFT calculations. Two new ESIPT cyanine dyes, namely (E)-4-(3-(benzo[d]thiazol-2-yl)-2-hydroxystyryl)-7-(dimethylamino)-2-phenyl chromenylium (PSS) and (E)-4-(3-(benzo[d]oxazol-2-yl)-2-hydroxystyryl)-7-(dimethylamino)-2-phenylchromenylium (PSO) were designed and fully studies. This is concerned with studying changes in intramolecular hydrogen bonds, molecular orbitals at the frontier of the ESIPT process, absorption and fluorescence spectra, and excited state energy barriers. As a result, both the systems considered here can undergo an ultrafast ESIPT reaction with PSS and then PSO. Furthermore, ESIPT is more accessible in the normal enol-form first excited singlet (S
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