Revisiting Anti-Stokes Emission Features of DNA-Stabilized Silver Nanoclusters.

 0 Người đánh giá. Xếp hạng trung bình 0

Tác giả: Cecilia Cerretani, Mikkel Baldtzer Liisberg, Giacomo Romolini, Vanessa Rück, Tom Vosch

Ngôn ngữ: eng

Ký hiệu phân loại: 770.11 Inherent features

Thông tin xuất bản: United States : ACS omega , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 683020

DNA-stabilized silver nanoclusters (DNA-AgNCs) are a class of fluorophores with interesting photophysical properties. They are capable of generating anti-Stokes fluorescence upon excitation with near-infrared lasers. The anti-Stokes fluorescence has previously been speculated to be either the result of consecutive photon absorption (upconversion) or hot band absorption (HBA). Here, we revisit the anti-Stokes fluorescence of DNA-AgNCs to determine the underlying mechanistic origin. We investigate two previously studied DNA-AgNCs together with two organic fluorophores with absorption and emission features in the same spectral regions as the DNA-AgNCs. From the recorded anti-Stokes fluorescence excitation spectra, we find that all the emitters exhibit an exponential-like decaying slope on the red side of the lowest energy absorption band. Furthermore, excitation power dependency measurements at different excitation wavelengths verify the one-photon nature of the anti-Stokes fluorescence. Ultimately, the lack of discrete optical transition features in the anti-Stokes fluorescence excitation spectra suggests that the HBA mechanism is the most plausible cause for the anti-Stokes fluorescence of the investigated DNA-AgNCs.
Tạo bộ sưu tập với mã QR

THƯ VIỆN - TRƯỜNG ĐẠI HỌC CÔNG NGHỆ TP.HCM

ĐT: (028) 36225755 | Email: tt.thuvien@hutech.edu.vn

Copyright @2024 THƯ VIỆN HUTECH