Robust half-metallic properties in two-dimensional CuCr₂Se₂X₂ (X = Cl, Br, I).

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Tác giả: Yanfeng Ge, Yujing Guo, Shuai Liu, Yong Liu, Yiran Peng, Wenhui Wan, Haimei Zhou

Ngôn ngữ: eng

Ký hiệu phân loại: 133.594 Types or schools of astrology originating in or associated with a

Thông tin xuất bản: England : Journal of physics. Condensed matter : an Institute of Physics journal , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 685359

In recent years, the rapid development of two-dimensional magnetic materials has revolutionized the field of spintronics, driven by their unique ability to combine magnetism and electronic functionality at the atomic scale. Here, we investigate the monolayer CuCr2Se2X2 (X = Cl, Br, I), which exhibit robust ferromagnetic (FM) behavior and half-metallicity with 100% spin polarization. The strong FM coupling, mediated by superexchange interactions, is rooted in the unique electronic structure of the Cr d-orbitals. Our findings reveal high Curie temperatures (TC) exceeding room temperature, with the Br variant achieving a remarkable 586 K. These exceptional properties, including the ability to modulate exchange interactions through strain engineering, highlight CuCr2Se2X2 as a versatile platform for flexible, high-performance spintronic devices, paving the way for advancements in next-generation electronic applications.
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