Observation of an Associative State in Aqueous Hydroxide.

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Tác giả: Evanthia Chatzigeorgiou, Yitao Cui, Faris Gelmukhanov, Johan Gråsjö, Yoshihisa Harada, Victor Kimberg, Pavel Krasnov, Jun Miyawaki, Michael Odelius, Sergey P Polyutov, Jan-Erik Rubensson, Conny Såthe, Stephan Thürmer, Takashi Tokushima, Hans Jakob Wörner, Kosuke Yamazoe, Zhong Yin

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: United States : Journal of the American Chemical Society , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 686123

The dynamics of chemical reactions in solution are of paramount importance in fields ranging from biology to materials science. Because the hydrogen-bond network and proton dynamics govern the behavior of aqueous solutions, they have been the subject of numerous studies over the years. Here, we report the observation of a previously unknown associative state in the hydroxide ion that forms when a proton from a neighboring water molecule approaches the hydroxide ion, utilizing resonant inelastic soft X-ray scattering (RIXS) and quantum dynamical simulations. State-of-the-art theoretical analysis reveals state mixing in the electronically excited states between aqueous hydroxide ions and the solvent. Our results give new insights into chemical bonding and excited-state dynamics in the aqueous environment. This investigation of associative states opens up new pathways for spectroscopic studies of chemical reaction dynamics and lays the foundation for directly accessing dynamic proton exchange in solution.
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