Triazole Drives Hole Localization and Superoxide Radical Formation for Enhancive Photocatalytic Cascade Isomerization/C─C Bond Scission of Biomass to Lactic Acid.

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Tác giả: Jinshu Huang, Hu Li, Jie Li, Huan Liu, Shunmugavel Saravanamurugan, Junqi Wang, Yu Wen

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: Germany : Small (Weinheim an der Bergstrasse, Germany) , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 690309

Chemocatalytic synthesis of lactic acid (LA) from biomass sugars involves heat-absorbing multistep cascade reactions mediated by different active sites, often encountering unsatisfactory selectivity. Here, a hole-localized carbon nitride-based photocatalyst (C-CNN) is constructed by covalent binding of heptazine and triazole skeleton via C─N bonds and further conjugated interaction with activated carbon, achieving the complete conversion of various biomass sugars to LA (up to 98.6% selectivity) at room temperature for 2 h. The introduced triazole electron donor in C-CNN can not only enhance the adsorption of sugar for the enhanced aldose-to-ketose isomerization over the localized hole (Lewis acid) on the triazole skeleton, but also modulate the valence band oxidation to circumvent the formation of •OH but only •O
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