Large Guest Molecules Selectively Forming sII- or sH-Type Hydrates: Chameleon-Like Behavior.

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Tác giả: Jiwoong Seol

Ngôn ngữ: eng

Ký hiệu phân loại: 027.68 *Libraries for nonprofit organizations

Thông tin xuất bản: United States : The journal of physical chemistry letters , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 691868

Over the past decades, extensive research on large guest molecules (LGMs) has shown that a given LGM exclusively forms only a single type of clathrate hydrate (sI, sII, or sH). This study challenges this prevailing understanding by revealing that certain LGMs can selectively form sII- or sH-type hydrates depending on the environment. This study presents various experimental evidence demonstrating that cyclohexylamine and cyclohexanol exhibit chameleon-like behavior, forming sII or sH hydrates when mixed with sII or sH formers, respectively. This intriguing structural modification induced by coguest inclusion is expected to broaden the scope of physicochemical investigations into hydrate materials. Furthermore, this study also suggests that shifting from the traditional approach, which has predominantly focused on single LGMs, could potentially drive breakthroughs in the development and application of sustainable hydrate-based technologies.
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