Balancing Electronic Spin State via Atomically-Dispersed Heteronuclear Fe-Co Pairs for High-Performance Sodium-Sulfur Batteries.

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Tác giả: Jordi Arbiol, Xiaoyu Bi, Andreu Cabot, Yapeng Cheng, Chen Huang, Canhuang Li, Hao Li, Junshan Li, Jiachen Ma, Ivan Pinto-Huguet, Yuchuan Ren, Jian Wang, Sen Xin, Dawei Yang, Jing Yu, Haining Zhang, Ruirui Zhao, Yingtang Zhou

Ngôn ngữ: eng

Ký hiệu phân loại: 583.67 *Ebenales, Primulales, Diapensiales, Thymelaeales (mezereum order)

Thông tin xuất bản: United States : Journal of the American Chemical Society , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 692065

Room-temperature sodium-sulfur (Na-S) batteries are emerging as a promising next-generation energy storage technology, offering high energy densities at low cost and utilizing abundant elements. However, their practical application is hindered by the shuttle effect of sodium-polysulfides and the sluggish kinetics of sulfur redox reactions. In this study, we demonstrate a heteronuclear diatomic catalyst featuring Fe and Co bimetallic sites embedded in nitrogen-doped hollow carbon nanospheres (Fe-Co/NC) as an effective sulfur host at the cathode of Na-S batteries. Aberration-corrected high-angle annular dark field scanning transmission electron microscopy demonstrates the presence of isolated Fe-Co atomic pairs, while synchrotron radiation X-ray absorption fine structure analysis confirms the (Fe-Co-N
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