Iron(III) Complexes with Luminescence Lifetimes of up to 100 ns to Enhance Upconversion and Photocatalysis.

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Tác giả: Isabelle Becker, Franc Meyer, Björn Pfund, Alessandro Prescimone, Joël Wellauer, Oliver S Wenger

Ngôn ngữ: eng

Ký hiệu phân loại: 582 Plants noted for specific vegetative characteristics and flowers

Thông tin xuất bản: United States : Journal of the American Chemical Society , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 692170

Iron is the most abundant transition metal element and would be the ideal replacement for noble metals in many applications that rely on luminescent and long-lived electronically excited states. We show that efficient reversible energy transfer between doublet excited states of iron complexes and triplet excited states on organic ligands improves energy storage by up to 350-fold. As a result, luminescence lifetimes of up to 100 ns are achieved, the upconversion from red to blue light becomes 68 times more efficient and the yield of benchmark photoredox reactions is significantly improved. These advances make iron coordination compounds more promising candidates for applications in lighting, solar energy conversion and photocatalysis.
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