Emestrin-type epipolythiodioxopiperazines from Aspergillus nidulans with cytotoxic activities by regulating PI3K/AKT and mitochondrial apoptotic pathways.

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Tác giả: Chunmei Chen, Aimin Fu, Pengkun Li, Qin Li, Changxing Qi, Wei Wei, Yang Xiao, Yonghui Zhang, Yuan Zhou, Hucheng Zhu

Ngôn ngữ: eng

Ký hiệu phân loại: 332.34 Pawnshops

Thông tin xuất bản: Germany : Natural products and bioprospecting , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 693596

Five novel emestrin-type epipolythiodioxopiperazines (ETPs), prenylemestrins C-G (1-5), along with two known ETPs, prenylemestrin A (6) and prenylemestrin B (7), were obtained from Aspergillus nidulans. Their structures were characterized by spectroscopic data, X-ray crystallographic data, ECD comparisons and calculations. Prenylemestrins C-G (1 - 5) represent a rare class of ETPs, characterized by a 2,5-dithia-7,9-diazabicyclo[4.2.2]decane-8,10-dione core involving a hemiterpene moiety. Notably, compound 6 exhibited moderate cytotoxicity, inducing G2/M cell cycle arrest and apoptosis of L1210 cells by regulating the PI3K/AKT signaling pathway and mitochondrial apoptotic mechanisms.
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