Effect of persulfate dosage on organic degradation using N-doped biochar: Reaction pathway and environmental implications.

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Tác giả: Jiawei Chen, Ruonan Duan, Yandi Hu, Shijia Li, Zhixiong Li, Wu Qin, Wei Tang, Tongshuai Wang, Jingqi Wu

Ngôn ngữ: eng

Ký hiệu phân loại: 133.594 Types or schools of astrology originating in or associated with a

Thông tin xuất bản: United States : Water environment research : a research publication of the Water Environment Federation , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 698420

Persulfate-based advanced oxidation processes (PS-AOPs) catalyzed by carbon-based catalysts are promising for removing organic pollutants via radical/non-radical pathways. However, the activation efficiency of peroxymonosulfate (PMS) or peroxydisulfate (PDS) usage and the reaction mechanism remain insufficiently understood. In this study, the effects of PMS/PDS dosage on the degradation of bisphenol A (BPA, 10 mg/L) were evaluated using N-doped biochar (N-BC, 0.2 g/L) assisted PS-AOPs. The reaction pathways were comprehensively investigated through a combination of characterization techniques and molecular simulations. With low PS dosages (0.05 and 0.1 mM), the degradation rate constants (
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