Recent research indicates that high-strength bolts could be more effectively and efficiently used to connect steel girders and fabricated decks or retrofit existing composite girders than headed studs. To reduce the number of bolt shear connectors and, thus, further accelerate the construction of composite girders, high-strength large bolts could be an excellent alternative, resulting in greater concrete stress below the bolt. Also, hybrid fiber-reinforced concrete (HFRC) has better tensile ductility and strength than that of ordinary concrete (OC). Therefore, this study tried to design eighteen push-out test specimens, including different configurations of bolt shear connectors, to investigate the static properties of post-installed, high-strength, large-bolt shear connectors with fabricated HFRC/OC slabs. The experimental results indicated that the capacity and initial stiffness of a high-strength large through-bolt shear connector was the smallest. The fiber might enhance the capacity and initial stiffness of bolt shear connectors. Increasing the bolt diameter can significantly enhance the initial stiffness and load-bearing capacity, while the clearance of the bolt hole had a great influence on the capacity, initial stiffness, and slippage of the post-installed high-strength large-bolt shear connector. Finally, the capacity equation and slip behavior of post-installed, high-strength, large-bolt shear connector with fabricated HFRC deck were obtained using the regression method, which could provide the reference for their design.