Unexpected 18-Fold Overlapped Feathery Fermi Pockets in Typical Thermoelectric Bi_{0.5}Sb_{1.5}Te_{3}.

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Tác giả: Wei Bai, Shengtao Cui, Mengruizhe Kong, Kai Li, Tongrui Li, Yi Liu, Zhanfeng Liu, Zhengming Shang, Zhe Sun, Yunbo Wu, Chong Xiao, Yi Xie, Chenxi Zhao

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: United States : Physical review letters , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 707664

Bi_{0.5}Sb_{1.5}Te_{3} is the most widely used p-type commercial thermoelectric materials over six decades, yet its complex electronic structure remains uncertain especially in band degeneracy and k_{z} dispersions. Here we show an unexpected band structure of 18-fold overlapped feathery Fermi pockets through substantial angle-resolved photoelectron spectroscopy data. Complemented with transport tests, we suggest that the high performance originates in the cooperation of four electronic features-momentum overlap of Fermi pockets, 18-fold band degeneracy, ultrasharp k_{y} dispersions, and heavy k_{z} bands. This cooperation of band features proposes a new paradigm for promising thermoelectrics.
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