Well-structured and ordered 2D layered semiconducting materials have excellent optical properties but limited advanced optoelectronic applications in their natural state. Altering their natural arrangement, through artificial heterostructures, strain and pressure engineering, chemical doping, intercalation, and alloying, can impart them with unusual optical properties and potentially enhance their performance in various applications. Among these approaches, alloying is generally difficult to control and disrupts the well-ordered homophilic crystal phase of these 2D crystals, albeit with the capability to control materials as thin as a single atomic layer. In this work, the synthesis of a low-dimension ordered-disordered layered 2D alloy of Mo