Phase-transfer-catalyst enabled enantioselective C-N coupling to access chiral boron-stereogenic BODIPYs.

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Tác giả: Luying Guo, Erhong Hao, Yuefei Hu, Lijuan Jiao, Zhong-Yuan Li, Xiao-Juan Lv, Juan Ma, Bin Su, Xue-Qing Zhang

Ngôn ngữ: eng

Ký hiệu phân loại: 583.43 *Minor orders of Hamamelididae

Thông tin xuất bản: England : Nature communications , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 724102

Tetracoordinate boron-based fluorescent materials have shown extensively applications in chemistry, biology and materials science owing to their unique optoelectronic properties. However, constructing chiral boron-stereogenic fluorophores through practical and universal strategies remains rare and challenging. Herein, as a proof of concept, we report an enantioselective postfunctionalization of boron dipyrromethene dyes (BODIPYs), to acess boron-stereogenic BODIPYs in moderate to good yields with commendable enantioselectivity. Chiral BODIPYs have attracted increasing attention owing to not only their distinctively photophysical properties and applications in circularly polarized luminescence (CPL) materials, but also diversely structural modification. In this·work, we present a phase-transfer-catalyst enabled enantioselective C-N coupling reaction of BODIPYs with diverse nucleophiles. This method serves as a practical S
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