Direct solid-phase nitrogenous fertilizer recovery from wastewater: The hybrid system of membrane contactor and solvent-driven fractional crystallization.

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Tác giả: Jong Kwon Choe, Yongju Choi, Younghun Kim, Changmin Lee, Dongwhan Lee, Jaebeom Park

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: England : Water research , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 738980

We propose a novel configuration that integrates a membrane contactor with solvent-driven fractional crystallization (SDFC) to recover ammonia from wastewater and produce it as solid-phase nitrogenous fertilizers. A liquid-gas membrane contactor strips ammonia from wastewater in a gaseous form, which enters a strip tank containing a binary mixture of an aqueous anion solution and an organic solvent. There, the ammonia reacts with anions, instantly protonating and forming solid-phase fertilizers. Batch SDFC experiments identified phosphate and sulfate as viable options for producing solid-phase fertilizers from the ammonia gas entering the strip tank. The hybrid system utilizing these acids produced high-grade fertilizers free from soil acidification concerns: a mixture of monoammonium phosphate and diammonium phosphate, and pure ammonium sulfate. Ammonium sulfate crystals in the strip tank grew epitaxially, representing a unique ammonium sulfate crystallization pattern when ammonium concentration gradually increased to supersaturation. A single system run produced solid fertilizers that amounted to 81.54 and 83.84% of the initially added phosphoric and sulfuric acid, respectively. Organic solvents in the strip tank could be recycled for at least five cycles while maintaining crystallization efficiencies of ≥82.63%. These results highlight the potential for semi-permanent operation of the system without the need for solvent replenishment.
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