Airborne microplastics pose a significant risk to human health. Similarly to the water-air transfer process, such as sea spray, aerosols generated during the wastewater treatment process, driven by aeration and mechanical agitation, are an overlooked potential source of airborne microplastics. This study constitutes the first attempt to investigate the pollution characteristics of microplastics in aerosols generated during wastewater treatment, based on laser direct infrared spectroscopy (LDIR) and pyrolysis-gas chromatography/mass spectrometry (Py-GC/MS). Microplastics were ubiquitously observed in aerosols from each unit of the wastewater treatment plant, with abundances in the range of 0.83-28.03 items·m