Environmentally Sustainable Hydrous Zirconium Oxide-Inulin as an Efficient Adsorbent for Ciprofloxacin Removal: Mechanistic and Thermodynamic Insights via Statistical Physics and Fractal-like Kinetic Modeling.

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Tác giả: Mahboob Alam, Monika Bharti, Mohd Nasir, Nafisur Rahman, Mohammad Shahzad Samdani

Ngôn ngữ: eng

Ký hiệu phân loại: 577.554 +Garden and household ecology

Thông tin xuất bản: United States : Langmuir : the ACS journal of surfaces and colloids , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 745369

Pharmaceutical pollutants like ciprofloxacin (CPF) pose environmental risks due to their persistence and limited removal by conventional treatment methods. To address this, a hydrous zirconium oxide-inulin (HZO-inulin) biomaterial was synthesized via wet precipitation and characterized using Fourier transform infrared spectroscopy (FT-IR), X-ray diffraction, thermogravimetric analysis-difference thermal analysis, X-ray photoelectron spectroscopy, Brunauer-Emmett-Teller surface area analysis, scanning electron microscopy-energy dispersive X-ray spectroscopy, and transmission electron microscopy. HZO-inulin exhibited high chemical stability under various aquatic conditions. CPF adsorption was optimized using the Box-Behnken design with a desirability function approach, achieving 99.28% removal and a maximum adsorption capacity of 181.46 mg/g under optimal conditions (adsorbent dose = 0.01 g, concentration = 85 mg/L, contact time = 35 min). Isotherm analysis using classical and statistical physics models revealed that the Freundlich model best fit the data, suggesting multilayer adsorption, while statistical physics model 2 indicated monolayer adsorption with two energy levels (
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