Thermally-induced covalent coupling of cobalt porphyrin molecules on Au(111).

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Tác giả: Carl Barthel, Mehdi Bouatou, Carmen J Calzado, Manuel Gruber, Nicolás Montenegro-Pohlhammer, Rocío Sánchez-de-Armas

Ngôn ngữ: eng

Ký hiệu phân loại: 536.2012 Heat transfer

Thông tin xuất bản: England : Journal of physics. Condensed matter : an Institute of Physics journal , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 745571

We investigated the thermally induced covalent coupling of cobalt porphyrin (CoP) molecules on an Au(111) surface using scanning tunnelling microscopy and first-principle calculations. While CoP molecules deposited at room temperature remain isolated due to electrostatic repulsion, annealing the substrate leads to their aggregation into chain-like structures with covalent bonding. Three distinct bonding motifs are identified, with calculations revealing weak magnetic coupling between theS=1/2Co ions. This work evidences a straightforward method for synthesising multinuclear complexes with magnetically coupled spins on surfaces, offering potential applications in molecular spintronics.
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