Nature-Inspired Nanoarray Catalyst toward Balanced Heat and Mass Transport in Photothermal Catalysis.

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Tác giả: Xingda An, Mujin Cai, Kai Feng, Le He, Chaoran Li, Hai Li, Shuang Liu, Jiahui Shen, Manzar Sohail, Valeri Tolstoy, Kewei Yu, Yuxuan Zhou, Zhijie Zhu

Ngôn ngữ: eng

Ký hiệu phân loại: 363.1063 Public safety programs

Thông tin xuất bản: United States : ACS nano , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 745605

Photothermal catalysis represents a clean, efficient, and sustainable approach to harnessing solar energy to drive chemical reactions. However, the inherent trade-off between mass and heat transport efficiencies poses significant challenges to its applicability. Herein, a nature-inspired hollow silica nanocone array catalyst (HSNCA/Co) is developed to address this limitation by enhancing the heat management and sunlight-absorptive ability, while maintaining the exposure of active sites. The nanocone array structure creates dual-flow-rate regions that enable the multidimensional optimization of thermal management and simultaneous mitigation of all three primary heat dissipation pathways. Moreover, the dense silica array enhances light trapping and plasmon coupling efficacy, achieving nearly 99% broadband absorption. In a CO
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